1. Otto Octavius aka Doctor Octopus
I swear they put so much detail into the cgi on his arms. There were a couple of scenes where I swore it was all real. I wanted arms just like Ock. They looked so cool. Alfred Molina portrayed thev character to a T and looked fantastic while doing it. The fight scenes with him were amaaing as well and the dialogue was perfect. "Oops, butterfingers."
2. Norman Osborn aka The Green Goblin
Now of course William Dafoe's portrayal was spot on. His Norman and his Goblin, too bad we didn't get to see more of Norman before he went Goblin and...ya know, died. But he perfectly pulled of that insane yet cunning business man. Remains the most faithful Live Action adaption of GG to date. Easily very memorable and very "Impressive!".
3. Flint Marko aka Sandman
Where do I start, easily the most emotionally moving villain. This scene, who can forget this scene
https://www.youtube.com/watch?v=rXOa5bWFRKw
The cgi was very detailed, the sand looked so real, and the Flint Marko costume green shirt and all was spot on comic to screen, copy n paste. The fight scenes done with the villain where visually impressive, now if only when he went giant he actually talked instead of roaring. Then again, when you're brain is basically shifting sand I guess there's a point where your mind goes a bit feral. But "What does it matter to you anyway"
4. Edward Brock Jr. aka Venom
Design wise very disappointing of course everyone is used to the more buff Venom. I'm guessing after the Ultimate Comics they thought they could go with a more sleek Venom actor which is understandable, but even then the symbiote made him look buff. But personality and general portrayl, I liked it. He may not have been as bulky but he was terrifying and he hated Peter just like in the comics for pretty much the same reasons too. So yeah, I think it did good. Not as good as some of the other villains but good. "If you know what I mean."
5. Harry Osborn aka New Goblin(Brace yourselves for this one folks)
Now while it would've made a bit more sense to me to bring in the Hobgoblin or another one of the Goblin impersonators/replacements and kept Harry a friend to Peter. This actually made sense, Harry had good reason to hate Spider-Man and after finding out Peter was Spidey, the man who practically stole the woman of his dreams also killed his father, it pushed him over the edge. Thus he wanted to kill Peter and became the New Goblin, the mask kinda looks like the Winter Soldier, the board was a cool concept, a bit too modernized, but cool nonetheless. Anyways I think it was done because there wasn't really away Peter without the Symbiote could defeat both Sandman and Venom two of his most powerful villains. So, he was always planned to do a complete turn and help Peter overcome the enemy. Death was unnecessary point blank though. Also, he got his head hit alot. Uhh, can't really think of a memorable quote for this on-*hits head on glider*
Well that's my outlook on the SM Franchise Villains. Clear as possible.