My vote is based not just on their appearance but their depth as characters. Gollum is the most complex character in LOTR and Neytiri is the best character in Avatar, and IMO they both have more emotional depth than characters like Optimus Prime or Davy Jones.
1. Gollum in Lord of the Rings Trilogy
2. T-Rex in Jurassic Park
3. King Kong in King Kong (2005)
4. Zoe Saladana/Sam Worthington's characters in Avatar
5. Monsters in Where the Wild Things Are
Honorable mention goes to Dr. Manhattan in Watchmen and Davy Jones in Pirates of the Caribbean sequels. Silver Surfer was pretty solid as well in Fantastic Four: Rise of the Silver Surfer
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